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B
only the entropy of the surroundings must increase
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C
either the entropy of the system or that of the surroundings must increase
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D
the total entropy of the system and the surroundings must increase
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Solution
The correct option is C the total entropy of the system and the surroundings must increase For a spontaneous reaction, the entropy of the universe should increase, i. e. total entropy of system and the surrounding must increase.